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- Jude Law as Sky Captain
- Gwyneth Paltrow as Polly Perkins
- Angelina Jolie as Franky Cook
- Giovanni Ribisi as Dex
- Michael Gambon as Editor Paley
- Omid Djalili as Kaji
- Bai Ling as The Mysterious Woman
- Julian Curry as Dr, Jorge Vargas
- Trevor Baxter as Dr. Walter Jennings
- Peter Law as Dr. Kessler
- Laurence Olivier as Dr. Totenkopf
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